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Time-Resolved Spectroscopy: An Experimental Perspective: Textbook Series in Physical Sciences

Autor Thomas Weinacht, Brett J. Pearson
en Limba Engleză Paperback – 31 mar 2021
This concise and carefully developed text offers a reader friendly guide to the basics of time-resolved spectroscopy with an emphasis on experimental implementation. The authors carefully explain and relate for the reader how measurements are connected to the core physical principles. They use the time-dependent wave packet as a building block for understanding quantum dynamics, progressively advancing to more complex topics. The topics are discussed in paired sections, one discussing the theory and the next presenting the related experimental methods.






A wide range of readers including students and newcomers to the field will gain a clear and practical understanding of how to measure aspects of molecular dynamics such as wave packet motion, intramolecular vibrational relaxation, and electron-electron coupling, and how to describe such measurements mathematically.


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Specificații

ISBN-13: 9780367780401
ISBN-10: 0367780402
Pagini: 372
Dimensiuni: 203 x 254 mm
Greutate: 0.45 kg
Ediția:1
Editura: CRC Press
Colecția CRC Press
Seria Textbook Series in Physical Sciences


Public țintă

Postgraduate and Undergraduate

Cuprins

Contents


Preface ix


Authors xi


Part I Introduction and Background 1


Chapter 1 Introduction 3


Chapter 2 Molecular Structure 11


Chapter 3 Light–Matter Interaction 41


Chapter 4 Introduction to Experimental Techniques 63


Part II Quantum Dynamics in One Dimension 73


Chapter 5 Field-Free Dynamics 75


Chapter 6 Field-Driven Dynamics 93


Part III Measurements of One Dimensional Dynamics 113


Chapter 7 Incoherent Measurements in 1D 115


Chapter 8 Coherent Optical Measurements in 1D 141


Chapter 9 Coherent Diffractive Measurements in 1D 165


Part IV Quantum Dynamics in Multiple Dimensions 183


Chapter 10 Explicit Approach to N-D Dynamics 185


Chapter 11 Implicit Approaches to N-D Dynamics 205


Part V Measurements of Multidimensional Dynamics 215


Chapter 12 Incoherent Measurements in ND 217


Chapter 13 Coherent Optical Measurements in ND 241


Chapter 14 Coherent Diffractive Measurements in ND 275


Chapter 15 One System, Multiple Approaches 283


Appendix A Quantum Mechanics Essentials 297


Appendix B Experimental Considerations 317


Appendix C Additional Problems 325


Bibliography 327


Index 337

Notă biografică

Thomas Weinacht is a Professor of Physics at Stony Brook University in New York.


He received his B.S. in physics from the University of Toronto 1995 and a Ph.D. in


physics from the University of Michigan in 2000. He started his position at Stony


Brook University in 2002. His research focuses on controlling and following molecular


dynamics with strong-field ultrafast laser pulses. He has published extensively


in both physics and chemistry journals, with an emphasis on interpreting experimental


measurements. His research group has developed a number of experimental techniques,


and he has organized multiple international conferences and workshops in the


field of time-resolved spectroscopy. He is a fellow of the American Physical Society.


 


Brett Pearson is an Associate Professor of Physics and Astronomy at Dickinson College


in Carlisle, PA. He obtained a B.A. in physics in 1997 from Grinnell College and


then a Ph.D. in physics from the University of Michigan in 2004. He was a postdoctoral


fellow at Stony Brook University before moving to his current position. At Dickinson,


Brett teaches across the curriculum and works with undergraduate students on


research related to both ultrafast pulse shaping and single-photon quantum mechanics.

Recenzii

"Weinacht and Pearson have produced a simple and direct introduction to the modern methods and motivations of ultrafast science, intended as a first text for students and scholars interested in this field. The chapter sections interleave physical concepts such as wave packets, correlated motion, or quantum tunneling with clear descriptions of the techniques that ultrafast optical scientists have developed in the last two decades, including the sources and tools of the trade. The result is an excellent introduction and practical guide to time resolved measurements."
--Philip H. Bucksbaum, Marguerite Blake Wilbur Chair and Professor of Photon Science, Applied Physics, and Physics, Stanford University
"How do I measure a ‘molecular movie’? Which observables do I obtain and how can they be interpreted? To answer these questions, a deeper understanding of the physics and the underlying models and assumptions, as well as the experimental techniques is essential. This is exactly the aim of this clearly written textbook. So far, no textbook exists that focuses on a time-dependent perspective accessible for both theoreticians and experimentalists. It succeeds in improving the common level of basic understanding of (quantum) dynamical models and experimental techniques…an excellent textbook"
--Prof. Dr. Stefanie Gräfe, Institute of Physical Chemistry, Abbe Center for Photonics, Jena University
 "An excellent, well-written and easy to read text. The approach is insightful, nicely blending intuitive physical pictures with sufficient mathematical formalism to enable calculations of real quantities of interest. The authors explain what information can be extracted from a variety of standard measurement techniques, including strengths and weaknesses of the various methods. I do not see a comparable book out there. I recommend it highly, not only for lecture courses on ultrafast spectroscopy and/or molecular dynamics, but as a primer for undergraduate and graduate students as they begin research projects in these areas. I intend to make it standard reading for students joining my group." --Robert R. Jones, Department Chair and Francis H. Smith Professor of Physics, University of Virginia

Descriere

This concise and carefully developed text offers a reader friendly guide to the basics of time-resolved spectroscopy with an emphasis on experimental implementation. The authors carefully explain and relate for the reader how measurements are connected to the core physical principles.