Chemistry in Action: Making Molecular Movies with Ultrafast Electron Diffraction and Data Science: Springer Theses
Autor Lai Chung Liuen Limba Engleză Paperback – 12 sep 2021
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Specificații
ISBN-13: 9783030548537
ISBN-10: 3030548538
Ilustrații: XX, 239 p. 110 illus., 106 illus. in color.
Dimensiuni: 155 x 235 mm
Greutate: 0.37 kg
Ediția:1st ed. 2020
Editura: Springer International Publishing
Colecția Springer
Seria Springer Theses
Locul publicării:Cham, Switzerland
ISBN-10: 3030548538
Ilustrații: XX, 239 p. 110 illus., 106 illus. in color.
Dimensiuni: 155 x 235 mm
Greutate: 0.37 kg
Ediția:1st ed. 2020
Editura: Springer International Publishing
Colecția Springer
Seria Springer Theses
Locul publicării:Cham, Switzerland
Cuprins
Chapter1: Introduction.- Chapter2: Methods: Experimental Techniques and Data Science.- Chapter3: Ultrafast Structural Dynamics of (EDO-TTF)2X.- Chapter4: Photocyclization Dynamics of Diarylethene.- Chapter5: Photoinduced Spin Crossover in Iron(II) Systems.- Chapter6: Future Work.- Chapter7: Conclusion.
Notă biografică
Dr. Lai Chung Liu received his PhD from the University of Toronto in 2019.
Textul de pe ultima copertă
The thesis provides the necessary experimental and analytical tools to unambiguously observe the atomically resolved chemical reactions. A great challenge of modern science has been to directly observe atomic motions during structural transitions, and while this was first achieved through a major advance in electron source brightness, the information content was still limited and new methods for image reconstruction using femtosecond electron diffraction methods were needed. One particular challenge lay in reconciling the innumerable possible nuclear configurations with the observation of chemical reaction mechanisms that reproducibly give the same kind of chemistry for large classes of molecules. The author shows that there is a simple solution that occurs during barrier crossing in which the highly anharmonic potential at that point in nuclear rearrangements couples high- and low-frequency vibrational modes to give highly localized nuclear motions, reducing hundreds of potentialdegrees of freedom to just a few key modes. Specific examples are given in this thesis, including two photoinduced phase transitions in an organic system, a ring closure reaction, and two direct observations of nuclear reorganization driven by spin transitions. The emerging field of structural dynamics promises to change the way we think about the physics of chemistry and this thesis provides tools to make it happen.
Caracteristici
Nominated as an outstanding PhD thesis by the University of Toronto Includes an accessible introduction to transient absorption spectroscopy, ultrafast electron diffraction, and related data science techniques Describes a groundbreaking process for the direct observation of atoms and molecules undergoing chemical reactions